For the younger grades (kindergarten through third grade) project we made "Pop Art Hearts" by using warm colors (reds, oranges, pinks) and cool colors (blues, greens, purples).
I taught the kids about warm and cool colors and then had them create two pop masterpieces using oil pastels on white construction paper. For their first piece, they created a heart and used at least three warm colors inside it. Then they used at least three cool colors on the outside. If they had time, they made a second piece, using the same techniques, but by flipping the colors (cool on the inside and warm on the outside).
When they were done, some of them used a dark color (dark blue, purple or black works well), to outline their heart, making it "pop" even more.